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Energy-transfer processes in Yb:Tm-doped KY3F10, LiYF4, and BaY2F8 single crystals for laser operation at 1.5 and 2.3 μm

Identifieur interne : 002215 ( Main/Exploration ); précédent : 002214; suivant : 002216

Energy-transfer processes in Yb:Tm-doped KY3F10, LiYF4, and BaY2F8 single crystals for laser operation at 1.5 and 2.3 μm

Auteurs : A. Braud [France, Russie] ; S. Girard [France] ; J. L. Doualan [France] ; M. Thuau [France] ; R. Moncorge [France] ; A. M. Tkachuk [France]

Source :

RBID : Pascal:00-0089039

Descripteurs français

English descriptors

Abstract

Energy-transfer processes have been quantitatively studied in various Tm:Yb-doped fluoride crystals. A comparison between the three host crystals which have been examined (KY3F10, LiYF4, and BaY2F8) shows clearly that the efficiency of the Yb→Tm energy transfers is larger in KY3F10 than in LiYF4 or BaY2F8. The dependence of the energy-transfer parameters upon the codopant concentrations has been experimentally measured and compared with the results calculated on the basis of migration-assisted energy-transfer models. Using these energy-transfer parameters and a rate equation model, we have performed a theoretical calculation of the laser thresholds for the 3H43F4 and 3H43H5 laser transitions of the Tm ion around 1.5 and 2.3 μm, respectively. Laser experiments performed at 1.5 μm in Yb:Tm:LiYF4 then led to laser threshold values in good agreement with those derived theoretically. Based on these results, optimized values for the Yb and Tm dopant concentrations for typical values of laser cavity and pump modes were finally derived to minimize the threshold pump powers for the laser transitions around 1.5 and 2.3 μm.


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Le document en format XML

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<sub>10</sub>
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<sub>2</sub>
F
<sub>8</sub>
single crystals for laser operation at 1.5 and 2.3 μm</title>
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<term>Band structure</term>
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<term>Experimental study</term>
<term>Impurity states</term>
<term>Lithium compounds</term>
<term>Potassium compounds</term>
<term>Solid state lasers</term>
<term>Theoretical study</term>
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<term>Potassium composé</term>
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<front>
<div type="abstract" xml:lang="en">Energy-transfer processes have been quantitatively studied in various Tm:Yb-doped fluoride crystals. A comparison between the three host crystals which have been examined (KY
<sub>3</sub>
F
<sub>10</sub>
, LiYF
<sub>4</sub>
, and BaY
<sub>2</sub>
F
<sub>8</sub>
) shows clearly that the efficiency of the Yb→Tm energy transfers is larger in KY
<sub>3</sub>
F
<sub>10</sub>
than in LiYF
<sub>4</sub>
or BaY
<sub>2</sub>
F
<sub>8</sub>
. The dependence of the energy-transfer parameters upon the codopant concentrations has been experimentally measured and compared with the results calculated on the basis of migration-assisted energy-transfer models. Using these energy-transfer parameters and a rate equation model, we have performed a theoretical calculation of the laser thresholds for the
<sup>3</sup>
H
<sub>4</sub>
<sup>3</sup>
F
<sub>4</sub>
and
<sup>3</sup>
H
<sub>4</sub>
<sup>3</sup>
H
<sub>5</sub>
laser transitions of the Tm ion around 1.5 and 2.3 μm, respectively. Laser experiments performed at 1.5 μm in Yb:Tm:LiYF
<sub>4</sub>
then led to laser threshold values in good agreement with those derived theoretically. Based on these results, optimized values for the Yb and Tm dopant concentrations for typical values of laser cavity and pump modes were finally derived to minimize the threshold pump powers for the laser transitions around 1.5 and 2.3 μm.</div>
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